High-quality, fully compressively strained CVD-grown GeSn multi-layers are produced with defects confinement near the Ge buffer/Si interface. With the Ge layers used as sacrificial layers, the optimum ultrasonic-assisted H2O2 etching technique, the low thermal budget gate stack (400 °C), and the S/D parasitic resistance reduction, the first stacked 3-Ge0.93Sn0.07-nanosheets pGAAFET with LCH = 60 nm achieved record high Ion=1975μA/μm per channel width among all GeSn pFETs. Uniform stacked GeSn nanosheet GAAFETs with low surface roughness are compatible with Si technologies and are good candidates for future technology nodes to extend Moore’s law for CMOS scaling.